Based on the first round of survey dataset from China Panel Study of Entrepreneurial Dynamics (CPSED) and according to the entrepreneurs with different aspiration, this paper compares the differences of entrepreneurial behaviors; explores the role of the growth aspiration in the new venture creation. This paper finds that: (i) for the way of opportunities identification, the growth-oriented entrepreneurs use more “fortuitous discovery” than the comfortable size entrepreneurs and growth aspiration is relevant to the way of opportunities identification; (ii) the growth-oriented entrepreneurs do more planning activities than the comfortable size entrepreneurs; (iii) the growth-oriented entrepreneurs do more resource acquisitions activities than the entrepreneurs preferring appropriate size. This paper shows that growth aspiration plays an important role in the new venture creation.